Directional sensing based on flexible aligned carbon nanotube film nanocomposites

作者:Sui, Chao; Yang, Yingchao; Headrick, Robert J.; Pan, Zixuan; Wu, Jianyang; Zhang, Jing; Jia, Shuai; Li, Xinwei; Gao, Weilu; Dewey, Oliver S.; Wang, Chao*; He, Xiaodong; Kono, Junichiro; Pasquali, Matteo; Lou, Jun*
来源:Nanoscale, 2018, 10(31): 14938-14946.
DOI:10.1039/c8nr02137f

摘要

The electrical behaviors under mechanical deformation of an aligned single-walled carbon nanotube (SWCNT) film nanocomposite have been systematically investigated in this work. Electrical signals along the CNT axis (parallel to) and perpendicular to the CNT axis (perpendicular to) follow a specific pattern, which enables the mechanical motion to be determined by vector analysis of such signals. The unique electrical behaviors of the sandwiched nanocomposites originate from the anisotropic characteristics of the CNT films. By combining in situ mechanical investigation with a coarse-grained molecular dynamics simulation, the shearing effect between SWCNTs is found to play a key role in stress-transfer along the parallel to direction, resulting in arc-shape cracks, while the peeling effect is dominant along the perpendicular to direction, leading to unifom SWCNT bar bridging at cracks. The fabricated CNT based sandwiched nanocomposite is believed to have great potential in building flexible all-direction sensors.