Size effects in ferroelectric thin films: 180 degrees domains and polarization relaxation

作者:Ahluwalia Rajeev*; Srolovitz David J
来源:Physical Review B, 2007, 76(17): 174121.
DOI:10.1103/PhysRevB.76.174121

摘要

The role of 180 degrees domain kinetics on size effects in ferroelectric thin films is studied within a time-dependent Ginzburg-Landau framework. The model incorporates the effect of the depolarization field by considering nonferroelectric-passive layers at the top and bottom surfaces. A critical length scale is predicted below which a depolarization field-induced spontaneous transition from a single domain to a 180 degrees domain pattern causes a time-dependent relaxation of the remnant polarization. This is consistent with the experiments by Kim [Phys. Rev. Lett. 95, 237602 (2005)], where a frequency dependence of the remnant polarization has indeed been observed.

  • 出版日期2007-11