US-DOE and CIAE international cooperation in age-dating uranium standards

作者：Treinen Kerri C.^*; Kinman William S.; Chen Yan; Zhu Liuchao; Cardon Annelise M. R.; Steiner Robert E.; Kayzar-Boggs Theresa M.; Williams Ross W.; Zhao Yong-Gang

来源：Journal of Radioanalytical and Nuclear Chemistry, 2017, 314(3): 2469-2474.

DOI：10.1007/s10967-017-5593-3

• Nuclear forensics
• Radiochronometry
• Multi-collector mass spectrometry
• Age-dating
• Thorium
• Uranium

In 2014 the United States Department of Energy and the China Institute of Atomic Energy collaborated in a study measuring the model ages of uranium certified reference materials. Lawrence Livermore National Laboratory (LLNL) and Los Alamos National Laboratory (LANL), and the Chinese Institute of Atomic Energy (CIAE) determined Th-230-U-234 model ages for uranium certified reference materials U010 and U850. The aim of this work was to collaborate with CIAE and compare methods for measuring the age of bulk uranium materials using the Th-230-U-234 radiochronometer. Accurate results for age-dating depend on the accurate calibration of the tracer materials (e.g., Th-229 and U-233) used for the isotope dilution mass spectrometry (IDMS) analyses. To facilitate inter-comparison of results, samples of a Th-230 standard reference material were distributed to each laboratory for Th-229 tracer inter-calibration. The resulting Th-230-U-234 model ages from this collaboration for U010 ranged from March 1956 to January 1959, which agree with the known material production date of June 5th, 1958. The determined model ages for U850 were from December 1955 to October 1957, which agree with the material production date of December 31, 1957. All three laboratories used independent methods to determine model ages for uranium standards that agree with known production ages and with previously reported results.

• 出版日期2017-12
• 单位Los Alamos; 中国原子能科学研究院