An efficient low-temperature route to nitrogen-doping and activation of mesoporous carbons for CO2 capture

作者：Huang, Kuan; Chai, Song-Hai^*; Mayes, Richard T.; Veith, Gabriel M.; Browning, Katie L.; Sakwa-Novak, Miles A.; Potter, Matthew E.; Jones, Christopher W.; Wu, You-Ting; Dai, Sheng

来源：Chemical communications, 2015, 51(97): 17261-17264.

DOI：10.1039/c5cc05619e

• DOPED MICROPOROUS CARBONS
• POROUS CARBONS
• CATALYTIC MATERIALS
• DIOXIDE CAPTURE
• ALKALI AMIDES
• SODIUM AMIDE
• ADSORPTION
• AMMONIA
• PERFORMANCE
• NITRIDATION

An innovative strategy for post-synthesis nitrogen-doping of mesoporous carbons (MCs) with high yields (> 90%) at low temperatures (230-380 degrees C) by using a strong base, sodium amide (NaNH2), was developed. The as-prepared N-doped MCs exhibit a significantly enhanced CO2 adsorption performance in terms of capacity and selectivity when compared to their parent MCs.

• 出版日期2015-12-18
• 单位南京大学