Elucidating the Origin of Anomalous Diffusion in Crowded Fluids

作者:Szymanski Jedrzej*; Weiss Matthias
来源:Physical Review Letters, 2009, 103(3): 038102.
DOI:10.1103/PhysRevLett.103.038102

摘要

Anomalous diffusion in crowded fluids, e.g., in the cytoplasm of living cells, is a frequent phenomenon. So far, however, the associated stochastic process, i.e., the propagator of the random walk, has not been uncovered. Here we show by means of fluorescence correlation spectroscopy and simulations that the properties of crowding-induced subdiffusion are consistent with the predictions for fractional Brownian motion or obstructed (percolationlike) diffusion, both of which have stationary increments. In contrast, our experimental results cannot be explained by a continuous time random walk with its distinct non-Gaussian propagator.

  • 出版日期2009-7-17