Two-Quantum Many-Body Coherences in Two-Dimensional Fourier-Transform Spectra of Exciton Resonances in Semiconductor Quantum Wells

作者:Karaiskaj Denis*; Bristow Alan D; Yang Lijun; Dai Xingcan; Mirin Richard P; Mukamel Shaul; Cundiff Steven T
来源:Physical Review Letters, 2010, 104(11): 117401.
DOI:10.1103/PhysRevLett.104.117401

摘要

We present experimental coherent two-dimensional Fourier-transform spectra of Wannier exciton resonances in semiconductor quantum wells generated by a pulse sequence that isolates two-quantum coherences. By measuring the real part of the signals, we determine that the spectra are dominated by two-quantum coherences due to mean-field many-body interactions, rather than bound biexcitons. Simulations performed using dynamics controlled truncation agree with the experiments.

  • 出版日期2010-3-19