Doping dependence of femtosecond quasiparticle relaxation dynamics in Ba(Fe,Co)(2)As-2 single crystals: Evidence for normal-state nematic fluctuations

作者：Stojchevska L^*; Mertelj T; Chu Jiun Haw; Fisher Ian R; Mihailovic D

来源：Physical Review B, 2012, 86(2): 024519.

DOI：10.1103/PhysRevB.86.024519

We systematically investigate the photoexcited (PE) quasiparticle (QP) relaxation and low-energy electronic structure in electron doped Ba(Fe1-xCox)(2)As-2 single crystals as a function of Co doping, 0 <= x <= 0.11. The evolution of the photoinduced reflectivity transients with x proceeds with no abrupt changes. In the orthorhombic spin-density-wave (SDW) state, a bottleneck associated with a partial charge-gap opening is detected, similar to previous results in different SDW iron pnictides. The relative charge gap magnitude 2 Delta(0)/k(B)T(s) decreases with increasing x. In the superconducting (SC) state, an additional relaxational component appears due to a partial (or complete) destruction of the SC state proceeding on a sub-0.5-picosecond timescale. From the SC component saturation behavior the optical SC-state destruction energy, U-p/k(B) = 0.3 K/Fe, is determined near the optimal doping. The subsequent relatively slow recovery of the SC state indicates clean SC gaps. The T dependence of the transient reflectivity amplitude in the normal state is consistent with the presence of a pseudogap in the QP density of states. The polarization anisotropy of the transients suggests that the pseudogap-like behavior might be associated with a broken fourfold rotational symmetry resulting from nematic electronic fluctuations persisting up to T similar or equal to 200 K at any x. The second moment of the Eliashberg function, obtained from the relaxation rate in the metallic state at higher temperatures, indicates a moderate electron phonon coupling, lambda less than or similar to 0.3, that decreases with increasing doping.

• 出版日期2012-7-19