Absence of a quantum limit to charge diffusion in bad metals

作者:Pakhira Nandan; McKenzie Ross H
来源:Physical Review B, 2015, 91(7): 075124.
DOI:10.1103/PhysRevB.91.075124

摘要

Good metals are characterized by diffusive transport of coherent quasiparticle states and the resistivity is much less than the Mott-Ioffe-Regel (MIR) limit, ha/e(2), where a is the lattice constant. In bad metals, such as many strongly correlated electron materials, the resistivity exceeds the Mott-Ioffe-Regel limit and the transport is incoherent in nature. Hartnoll, loosely motivated by holographic duality (AdS/CFT correspondence) in string theory, recently proposed a lower bound to the charge-diffusion constant, D greater than or similar to (h) over bar nu(2)(F)/(k(B)T), in the incoherent regime of transport, where nu(F) is the Fermi velocity and T the temperature. Using dynamical mean-field theory (DMFT) we calculate the charge-diffusion constant in a single band Hubbard model at half filling. We show that in the strongly correlated regime the Hartnoll's bound is violated in the crossover region between the coherent Fermi-liquid region and the incoherent (bad metal) local moment region. The violation occurs even when the bare Fermi velocity nu(F) is replaced by its low-temperature renormalized value nu(F)*. The bound is satisfied at all temperatures in the weakly and moderately correlated systems as well as in strongly correlated systems in the high-temperature region where the resistivity is close to linear in temperature. Our calculated charge-diffusion constant, in the incoherent regime of transport, also strongly violates a proposed quantum limit of spin diffusion, D-s similar to 1.3 (h) over bar /m, where m is the fermion mass, experimentally observed and theoretically calculated in a cold degenerate Fermi gas in the unitary limit of scattering.

  • 出版日期2015-2-23