Attoclock reveals natural coordinates of the laser-induced tunnelling current flow in atoms

作者：Pfeiffer, Adrian N.^*; Cirelli, Claudio; Smolarski, Mathias; Dimitrovski, Darko; Abu-samha, Mahmoud; Madsen, Lars Bojer; Keller, Ursula

来源：Nature Physics, 2012, 8(1): 76-80.

DOI：10.1038/nphys2125

• ATTOSECOND ANGULAR STREAKING
• ORDER HARMONIC-GENERATION
• RARE-GASES
• IONIZATION
• FIELD
• INTENSE
• PULSES
• DELAY

In the research area of strong-laser-field interactions and attosecond science(1), tunnelling of an electron through the barrier formed by the electric field of the laser and the atomic potential is typically assumed to be the initial key process that triggers subsequent dynamics(1-3). Here we use the attoclock technique(4) to obtain experimental information about the electron tunnelling geometry (the natural coordinates of the tunnelling current flow) and exit point. We confirm vanishing tunnelling delay time, show the importance of the inclusion of Stark shifts(5,6) and report on multi-electron effects clearly identified by comparing results in argon and helium atoms. Our combined theory and experiment allows us to single out the geometry of the inherently one-dimensional tunnelling problem, through an asymptotic separation of the full three-dimensional problem. Our findings have implications for laser tunnel ionization in all atoms and in particular in larger molecular systems with correspondingly larger dipoles and polarizabilities.

• 出版日期2012-1