Decadal changes in dissolved inorganic carbon in the Pacific Ocean

作者：Kouketsu Shinya^*; Murata Akihiko; Doi Toshimasa

来源：Global Biogeochemical Cycles, 2013, 27(1): 65-76.

DOI：10.1029/2012GB004413

Using high-quality data sets obtained about a decade apart, we examined the changes of dissolved inorganic carbon in the Pacific Ocean, separating anthropogenic and natural CO2. Observations along three transoceanic sections along 47 degrees N, 179 degrees E, and 17 degrees S showed both decadal increases (>20 mu mol kg(-1)) and decreases (<-20 mu mol kg(-1)) of anthropogenic CO2 in thermocline waters. As a result, the decadal-scale storage of anthropogenic CO2 north of 40 degrees N in the North Pacific was close to +/- 0mol m(-2) a(-1), except in the western subarctic Pacific. In contrast, in subtropical regions of both hemispheres, we found an increasing trend of >10 mu mol kg(-1) in oceanic uptake of anthropogenic CO2, reflecting accumulation in mode waters. Along 17 degrees S, increases of anthropogenic CO2 were >20 mu mol kg(-1), larger than expected from increases of anthropogenic CO2 in the atmosphere. The annual water-column inventories of anthropogenic CO2 changes calculated in 20 degrees longitudinal or 10 degrees latitudinal bands throughout the Pacific Ocean revealed relatively high values (>0.7mol m(-2) a(-1)) in the subtropical regions of both hemispheres and low values in the tropical Pacific. This distribution pattern is similar to previous estimates for the Anthropocene, implying that the redistribution processes of anthropogenic CO2 have not changed on a basin scale over the last decade. We estimated the total anthropogenic and natural CO2 storage in the Pacific Ocean to be 8.4 +/- 0.5 and 0.6 +/- 0.4 Pg carbon decade(-1), respectively.

• 出版日期2013