Droplet formation and scaling in dense suspensions

作者：Miskin Marc Z; Jaeger Heinrich M^*

来源：Proceedings of the National Academy of Sciences, 2012, 109(12): 4389-4394.

DOI：10.1073/pnas.1111060109

• particle packing
• contact angle
• irrotational flow
• jamming

When a dense suspension is squeezed from a nozzle, droplet detachment can occur similar to that of pure liquids. While in pure liquids the process of droplet detachment is well characterized through self-similar profiles and known scaling laws, we show here the simple presence of particles causes suspensions to break up in a new fashion. Using high-speed imaging, we find that detachment of a suspension drop is described by a power law; specifically we find the neck minimum radius, r(m), scales like tau(2/3) near breakup at time tau = 0. We demonstrate data collapse in a variety of particle/liquid combinations, packing fractions, solvent viscosities, and initial conditions. We argue that this scaling is a consequence of particles deforming the neck surface, thereby creating a pressure that is balanced by inertia, and show how it emerges from topological constraints that relate particle configurations with macroscopic Gaussian curvature. This new type of scaling, uniquely enforced by geometry and regulated by the particles, displays memory of its initial conditions, fails to be self-similar, and has implications for the pressure given at generic suspension interfaces.

• 出版日期2012-3-20