Attosecond Streaking of Correlated Two-Electron Transitions in Helium

作者:Pazourek Renate*; Feist Johannes; Nagele Stefan; Burgdoerfer Joachim
来源:Physical Review Letters, 2012, 108(16): 163001.
DOI:10.1103/PhysRevLett.108.163001

摘要

We present fully ab initio simulations of attosecond streaking for ionization of helium accompanied by shakeup of the second electron. This process represents a prototypical case for strongly correlated electron dynamics on the attosecond time scale. We show that streaking spectroscopy can provide detailed information on the Eisenbud-Wigner-Smith time delay as well as on the infrared-field dressing of both bound and continuum states. We find a novel contribution to the streaking delay that stems from the interplay of electron-electron and infrared-field interactions in the exit channel. We quantify all the contributions with attosecond precision and provide a benchmark for future experiments.

  • 出版日期2012-4-20