Stability of spin-driven ferroelectricity in the thin-film limit: Coupling of magnetic and electric order in multiferroic TbMnO3 films

作者:Glavic Artur*; Becher Carsten; Voigt Joerg; Schierle Enrico; Weschke Eugen; Fiebig Manfred; Brueckel Thomas
来源:Physical Review B, 2013, 88(5): 054401.
DOI:10.1103/PhysRevB.88.054401

摘要

We demonstrate spin-spiral-induced ferroelectricity in epitaxial TbMnO3 films grown on YAlO3 substrates down to a film thickness of 6nm. The ferroelectric polarization is identified by optical second-harmonic generation. Using x-ray resonant magnetic scattering we directly prove the existence of a noncollinear magnetic structure in the ferroelectric phase and thus bulk-like multiferroicity. The electric-field-induced reversal of the magnetic domains along with the reversal of the ferroelectric polarization evidences the rigid coupling of magnetic and ferroelectric order and hence a "giant" magnetoelectric effect in the films.

  • 出版日期2013-8-1