Nuclear magnetic resonance at up to 10.1 GPa pressure detects an electronic topological transition in aluminum metal

作者:Meissner Thomas*; Goh Swee K; Haase Juergen; Richter Manuel; Koepernik Klaus; Eschrig Helmut
来源:Journal of Physics: Condensed Matter , 2014, 26(1): 015501.
DOI:10.1088/0953-8984/26/1/015501

摘要

High-sensitivity Al-27 nuclear magnetic resonance (NMR) measurements of aluminum metal under hydrostatic pressure of up to 10.1 GPa reveal an unexpected negative curvature in the pressure dependence of the electronic density of states measured through shift and relaxation, which violates free electron behavior. A careful analysis of the Fermiology of aluminum shows that pressure induces an electronic topological transition (Lifshitz transition) that is responsible for the measured change in the density of states. The experiments also reveal a sudden increase in the NMR linewidth above 4.2 GPa from quadrupole interaction, which is not in agreement with the metal's cubic symmetry.

  • 出版日期2014-1-8