Artificial Photosynthesis: Porphyrin/SiO2/Cp*Rh(bpy)Cl Hybrid Nanoparticles Mimicking Chloroplast with Enhanced Electronic Energy Transfer for Biocatalyzed Artificial Photosynthesis (Adv. Funct. Mater. 9/2018)

作者：Xiaoyuan Ji; Jie Wang; Lin Mei; Wei Tao; Austin Barrett; Zhiguo Su; Shaomin Wang; Guanghui Ma; Jinjun Shi; Songping Zhang

来源：Advanced Functional Materials, 2018, 28(9): n/a-n/a.

DOI：10.1002/adfm.201870061

• artificial photosynthesis
• chloroplast mimicks
• intermolecular electron transfer
• intramolecular electron transfer
• sol–gel reactions

In article number 1705083, Jinjun Shi, Songping Zhang, and co‐workers present an integrated artificial photosynthesis system mimicking the structure and function of photosynthesis process performed by chloroplasts in green plants. Upon light irradiation, photo‐induced electrons transfer from a photosensitizer via an electron mediator to an oxidized coenzyme for its regeneration to NADH, which can provide reduction power for enzymatic conversion of CO2 to formic acid.

• 出版日期2018
• 单位Harvard Medical School; 中国科学院大学; 郑州大学; Brigham and Women's Hospital; Harvard medical school; harvard medical school; 中山大学