科研之友
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摘要
Light-absorbing, atmospheric particles have gained greater attention in recent years because of their direct and indirect impacts on regional and global climate. Atmospheric black carbon (BC) aerosol is a leading climate warming agent, yet uncertainties in the global direct aerosol radiative forcing remain large. Based on a year of aerosol absorption measurements at seven wavelengths, BC concentrations were investigated in Dhanbad, the coal capital of India. Coal is routinely burned for cooking and residential heat as well as in small industries. The mean daily concentrations of ultraviolet-absorbing black carbon measured at 370 nm (UVBC) and black carbon measured at 880 nm (BC) were 9.8 +/- 5.7 and 6.5 +/- 3.8 mu g m(-3), respectively. The difference between UVBC and BC, Delta-C, is an indicator of biomass or residential coal burning and averaged 3.29 +/- 4.61 mu g m(-3). An alternative approach uses the Angstrom Exponent (AE) to estimate the biomass/coal and traffic BC concentrations. Biomass/coal burning contributed similar to 87% and high temperature, fossil-fuel combustion contributed similar to 13% to the annual average BC concentration. The post-monsoon seasonal mean UVBC values were 10.9 mu g m(-3) and BC of 7.2 mu g m(-3). Potential source contribution function analysis showed that in the post-monsoon season, air masses came from the central and northwestern Indo-Gangetic Plains where there is extensive agricultural burning. The mean winter UVBC and BC concentrations were 15.0 and 10.1 mu g m(-3), respectively. These higher values were largely produced by local sources under poor dispersion conditions. The direct radiative forcing (DRF) due to UVBC and BC at the surface (SUR) and the top of the atmosphere (TOA) were calculated. The mean atmospheric heating rates due to UVBC and BC were estimated to be 1.40 degrees K day(-1) and 1.18 degrees K day(-1), respectively. This high heating rate may affect the monsoon circulation in this region.
- 出版日期2018-2-15
