Multiple Length Scale Instabilities of Unidirectional Pulse Propagation in a Diffusion-Fed Gel

作者:Lu, Xing-Jie; Ren, Lin; Gao, Qing-Yu; Yang, Ying-Ying; Zhao, Yue-Min; Huang, Jun; Lv, Xiao-Li; Epstein, Irving R.*
来源:Journal of Physical Chemistry Letters, 2013, 4(22): 3891-3896.
DOI:10.1021/jz402117m

摘要

Patterns containing multiple length scales arise in a variety of natural systems such as lateral veins in leaves, fingerprints, wrinkled skin, and dendritic crystals. Here we observe period-doubling and bursting instabilities in the spatial extent of wave propagation in a gel-filled capillary tube open at one end and containing the Belousov-Zhabotinsky (BZ) reaction-diffusion system. We analyze the relationship between the multiple propagation distances of pulse waves and the local kinetics of the reaction-diffusion system. Simulations with a five-variable Oregonator model qualitatively mimic the multiple length scale patterns of pulse propagation observed in our experiments, suggesting that the study of these phenomena in reaction-diffusion systems may be helpful in understanding complex multiple length scale dynamical behaviors in nature.