Fabrication of AI GaN nanorods with different AI compositions for emission enhancement in UV range

作者:Dai, Jiangping; Liu, Bin*; Zhuang, Zhe; He, Guotang; Zhi, Ting; Tao, Tao; Xu, Qingjun; Li, Yi; Ge, Haixiong; Xie, Zili; Zhang, Rong*
来源:Nanotechnology, 2017, 28(38): 385205.
DOI:10.1088/1361-6528/aa7ba4

摘要

Highly ordered AlxGa1-xN nanorods with varied aluminum alloy compositions (0.18 <= x <= 0.8) are fabricated with nanoimprint lithography and top-down dry etching techniques. And the structural properties and morphology are obtained by scanning electron microscopy (SEM) and transmission electron microscopy (TEM). Compared with as-grown AlGaN samples, nanorod samples reveal outstanding optical performance on account of strain releasing and light extraction enhancement. Through Raman scattering and cathodeluminescence measurements, it has been observed clear redshifts of E(2)h modes and near band edge emission (NBE) peaks of AlGaN nanorods compared to the planar ones, indicating the residual strain releasing after nano-fabrication. The integrated intensities of NBE peaks of AlGaN nanorods manifest light emission enhancement up to 2.7 at deep-UV range. Finite-difference time-domain (FDTD) simulations have been adopted to investigate the light extraction and far-field distribution of such structures, it turned out that ordered nanorod array can enhance the TM polarized emission extraction 2-7 folds compared to the planar structure. The optical regulation in nanorod arrays should take the responsibility for the observed optical enhancements, which is proved by the far-field distribution of light, thus it can improve the performance of ultraviolet LEDs.