A room temperature low-threshold ultraviolet plasmonic nanolaser

作者：Zhang, Qing; Li, Guangyuan; Liu, Xinfeng; Qian, Fang; Li, Yat; Sum, Tze Chien; Lieber, Charles M.^*; Xiong, Qihua

来源：Nature Communications, 2014, 5(1): 4953.

DOI：10.1038/ncomms5953

• NANOWIRE LASERS
• WAVE-GUIDES
• GAIN

Constrained by large ohmic and radiation losses, plasmonic nanolasers operated at visible regime are usually achieved either with a high threshold (10(2)-10(4) MW cm(-2)) or at cryogenic temperatures (4-120 K). Particularly, the bending-back effect of surface plasmon (SP) dispersion at high energy makes the SP lasing below 450 nm more challenging. Here we demonstrate the first strong room temperature ultraviolet (similar to 370 nm) SP polariton laser with an extremely low threshold (similar to 3.5 MW cm(-2)). We find that a closed-contact planar semiconductor-insulator-metal interface greatly lessens the scattering loss, and more importantly, efficiently promotes the exciton-SP energy transfer thus furnishes adequate optical gain to compensate the loss. An excitation polarization-dependent lasing action is observed and interpreted with a microscopic energy-transfer process from excitons to SPs. Our work advances the fundamental understanding of hybrid plasmonic waveguide laser and provides a solution of realizing room temperature UV nanolasers for biological applications and information technologies.

• 出版日期2014-9