Anisotropic exchange in LiCu2O2

作者:Seidov Z; Gavrilova T P; Eremina R M; Svistov L E; Bush A A; Loidl A; von Nidda H A Krug*
来源:PHYSICAL REVIEW B, 2017, 95(22): 224411.
DOI:10.1103/PhysRevB.95.224411

摘要

We investigate the magnetic properties of the multiferroic quantum-spin system LiCu2O2 by electron spin resonance (ESR) measurements at X-and Q-band frequencies in a wide temperature range (TN1 <= T <= 300 K). The observed anisotropies of the g tensor and the ESR linewidth in untwinned single crystals result from the crystal-electric field and from local exchange geometries acting on the magnetic Cu2+ ions in the zigzag-ladder-like structure of LiCu2O2. Supported by a microscopic analysis of the exchange paths involved, we show that both the symmetric anisotropic exchange interaction and the antisymmetric Dzyaloshinskii-Moriya interaction provide the dominant spin-spin relaxation channels in this material.

  • 出版日期2017-6-7