Nonadiabatic Effects in the Irradiation of Ethylene

作者:Wang, Zhi-Ping; Dinh, Phuong Mai*; Reinhard, Paul Gerhard; Suraud, Eric; Zhang, Feng Shou
来源:International Journal of Quantum Chemistry, 2011, 111(2): 480-486.
DOI:10.1002/qua.22656

摘要

In the framework of the time-dependent local density approximation, applied to valence electrons, coupled nonadiabatically to molecular dynamics of ions, the irradiations of ethylene by laser and fast charged projectiles are studied. We find that the Coulomb fragmentation sensitively depends on the laser frequency and on the charge of the projectile.