NOX reduction over paper-structured fiber composites impregnated with Pt/Al2O3 catalyst for exhaust gas purification

作者:Koga Hirotaka*; Ishihara Hirotake; Kitaoka Takuya; Tomoda Akihiko; Suzuki Ryo; Wariishi Hiroyuki
来源:Journal of Materials Science, 2010, 45(15): 4151-4157.
DOI:10.1007/s10853-010-4504-6

摘要

Pt/Al2O3 catalyst powder was successfully incorporated in a microstructured paper-like matrix composed of a ceramic fiber network, by use of a simple papermaking technique. As-prepared composite, denoted paper-structured catalyst, was applied to the reduction of nitrogen oxide (NOX) in the presence of propene, for exhaust gas purification. The paper-structured catalyst demonstrated higher NOX reduction efficiency and more rapid thermal responsiveness than a conventional Pt-loaded honeycomb catalyst, indicating that the paper-like structure with interconnected pore spaces contributes to effective transport of heat and reactants to the catalyst surfaces. Furthermore, the paper-structured catalyst with the appearance of flexible paperboard has a high degree of utility. The efficiency of utilization of Pt catalyst was improved by using hierarchically assembled paper-structured catalysts with preferential location of Pt catalyst in the upper part. The paper-structured catalyst composite with paper-like utility and porous microstructure is thought to be a promising catalytic material for efficient NOX gas purification.

  • 出版日期2010-8