Southwestern US Biomass Burning Smoke Hygroscopicity: The Role of Plant Phenology, Chemical Composition, and Combustion Properties

作者:Gomez S L; Carrico C M*; Allen C; Lam J; Dabli S; Sullivan A P; Aiken A C; Rahn T; Romonosky D; Chylek P; Sevanto S; Dubey M K*
来源:JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2018, 123(10): 5416-5432.
DOI:10.1029/2017JD028162

摘要

Biomass burning emissions have substantially increased with continued warming and drying in the southwestern U.S., impacting air quality and atmospheric processes. To better quantify impacts of biomass burning aerosols, an extensive laboratory study of fresh smoke emissions was conducted at Los Alamos National Laboratory. Laboratory burn experiments with selected native and invasive southwestern U.S. fuels were used to elucidate the role of fuel type, chemical composition, and ignition method on the hygroscopicity of smoke. Here we focus on a custom controlled relative humidity (RH) nephelometry system using the direct measurement of aerosol light scattering with two nephelometersone at dry conditions and one at a controlled high RH (RH similar to 85%). Aerosol hygroscopicity was highly variable with the enhancement in light scattering coefficient in the range of 1.02

  • 出版日期2018-5-27
  • 单位Los Alamos