Measurement of the Am-240 production cross section via proton irradiation of Pu-242

作者:Ellison Paul A; McLaughlin Joseph P; Stavsetra Liv; Gregorich Kenneth E; Nitsche Heino*
来源:Radiochimica Acta, 2014, 102(7): 561-568.
DOI:10.1515/ract-2014-2219

摘要

A new nuclear reaction for the production of Am-240 was experimentally investigated. Targets of 150-500 mu g/cm(2) Pu-242 on 2 mu mTi were produced through molecular deposition. Five irradiations, in which Pu-242, Ti-nat, and Ni-nat targets were jointly activated with protons from the Lawrence Berkeley National Laboratory 88-Inch Cyclotron produced Am-240, V-48, and Ni-57, respectively. The radioactive decay of these nuclides was monitored using high-purity Ge gamma ray detectors in the weeks following irradiation. A maximum Pu-242(p, 3n)Am-240 nuclear reaction cross section was measured to be 45 +/- 13 mb with 23 MeV protons. While this value is lower than theoretical predictions, it is high enough to be the most viable nuclear reaction for the large-scale production of Am-240.

  • 出版日期2014-7