AFM measurements of adhesive forces between carbonaceous particles and the substrates

作者：Zhang, Tianqi; Peng, Wei^*; Shen, Ke; Yu, Suyuan

来源：Nuclear Engineering and Design, 2015, 293: 87-96.

DOI：10.1016/j.nucengdes.2015.06.022

• NANOSCALE ROUGH SURFACES
• RESUSPENSION
• ENERGIES
• DEPOSITION
• CONTACT
• MODEL
• DUST
• HTR

Graphite dust is carbonaceous particles generated during operation of High Temperature Gas-Cooled Reactors (HTR). Graphite dust resuspension is the key behavior associated with HTR source term analyses and environmental safety assessment. The adhesive force is the key factor that determines the resuspension rate. The present study used an atomic force microscope (AFM) to measure the adhesive force between a single carbonaceous particle and the substrate. The measurements were performed on mica, graphite IG110 and Inconel 800H. The prepared "probe cantilevers" were mesocarbon microbeads (MCMB), fuel element debris from HTR-10 and graphite NBG18. The equivalent work of adhesion was derived from the measured adhesive force and calculated based on substrate profile approximation and the JKR theoretical model. The measured work was smaller than the ideal work of adhesion, most likely due to the rough particle morphology and the rough substrate surface. Additionally, a shape factor imposes a constraint on the lateral deformation of the particles. Furthermore, surface roughness could reduce the adhesive force some depending on the particle size. Once the particle was too small to be trapped into a trough, the adhesive force would not be further reduced.

• 出版日期2015-11
• 单位清华大学