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摘要
In this Perspective article we describe how the processes involving the redox shuttle-dye regeneration, recombination, and diffusion-affect the photovoltaic performance of dye-sensitized solar cells, DSSCs. Key literature on the mechanistically complicated, but ubiquitously employed, triiodide/iodide electrolyte is reviewed. Literature examples and recent results from our laboratory in utilizing one-electron outersphere redox shuttles in place of triiodide/iodide are then presented.
- 出版日期2011-2
