Ultranarrow Band Absorbers Based on Surface Lattice Resonances in Nanostructured Metal Surfaces

作者：Li Zhongyang; Butun Serkan; Aydin Koray^*

来源：ACS Nano, 2014, 8(8): 8242-8248.

DOI：10.1021/nn502617t

• plasmonics
• narrow band
• perfect absorption
• surface lattice resonance
• nanostructures
• ultrasensitive biosensing
• symmetry breaking

Nanostructured metals have received a significant amount of attention in recent years due to their exciting plasmonic and photonic properties enabling strong field localization, light concentration, and strong absorption and scattering at their resonance frequencies. Resonant plasmonic and metamaterial absorbers are of particular interest for applications in a wide variety of technologies including photothermal therapy, thermophotovoltaics, heat assisted magnetic recording, hot-electron collection, and biosensing. However, it is rather challenging to realize ultranarrow absorption bands using plasmonic materials due to large optical losses in metals that decrease the quality factor of optical resonators. Here, we theoretically and experimentally demonstrate an ultranarrow band absorber based on the surface lattice resonances (SIRS) in periodic nanowire and nanoring arrays on optically thick, reflecting metallic films. In experiments, we observed ultranarrow band resonant absorption peaks with a bandwidth of 12 nm and absorption amplitude exceeding 90% at visible frequencies. We demonstrate that the resonance absorption wavelength, amplitude of the absorption peak, and the bandwidth can be controlled by tuning the periodicity and the thickness of nanoring and nanowire arrays. Unlike conventional plasmonic absorbers utilizing common metal insulator metal stacks, our narrow band absorber consists solely of metals, facilitating stronger optical interaction between the SLR of periodic nanostructures and the highly reflective film. Moreover, by introducing asymmetry to the nanoring/nanowire hybrid system, we observe the spectral evolution of resonance splitting enabled by strong coupling between two individual SLRs arising from nanoring and nanowire arrays. Designing such all metallic nanostructure arrays is a promising route for achieving ultranarrow band absorbers which can be used as absorption filters, narrow band thermal emitters in thermophotovoltaics, and plasmonic biosensors.

• 出版日期2014-8
• 单位西北大学