摘要

An improved method, factor analysis with non-negative constraints (FA-NNC) was adopted to apportion the sources of sediment polycyclic aromatic hydrocarbons (PAHs) in Dalian Bay, China. Cosine similarity and Monte Carlo uncertainty analysis were used to assist the FA-NNC source resolution. The results identified three sources for PAHs, which were overall traffic, diesel engine emissions and residential coal combustion. The contributions of these sources were quantified as 78 4.6% from overall traffic, 12 3.2% from diesel engine emissions, and 10 1.9% from residential coal combustion. The results from the Monte Carlo uncertainty analysis indicated that the model was robust and convergent.