Historical Records of Mercury, Lead, and Polycyclic Aromatic Hydrocarbons Depositions in a Dated Sediment Core from the Eastern Mediterranean

作者：Azoury S; Tronczynski J^*; Chiffoleau J F; Cossa D; Nakhle K; Schmidt S; Khalaf G

来源：Environmental Science & Technology, 2013, 47(13): 7101-7109.

DOI：10.1021/es4005637

Depth profiles of mercury, lead and its stable isotopes, and polycyclic aromatic hydrocarbons were determined in a dated sediment core from the Levantine basin. Sedimentary records show that preindustrial fluxes and levels of Hg, Pb, and PAHs remained generally constant in the region before 1850. An almost concurrent uniform increase of both metals and PAHs deposition occurring at the beginning of the Industrial Revolution suggests coal combustion as a main source of these contaminants in the Levantine basin after the 1850s. However, none of the contaminant profiles indicates a decline after 1950-60, the characteristic period of coal use reduction. The modem fluxes of Hg and Pb reveal a 3- to 5-fold increase over preindustrial loads, while the contemporaneous flux of PAHs rises by 4-7 times. On the whole, records in the Eastern Mediterranean suggest atmospheric inputs from relatively distant sources, likely from Central and Eastern Europe.

• 出版日期2013-7-2